Nearly a decade later, they're reportedly ready for an onscreen reunion.
There's scant details about the project and no word on whether the couple, who have six kids together, would be up for a Mr. and Mrs. Smith 2. That film grossed more than $186 million at the domestic box office.
But Variety reported that Jolie had written the script herself. She and her husband will develop it together.
Celebrity Couples of 2014 [PHOTOS]